These are the following quotes from The Smurfs 2011 movie.
"There is a place. A place that knows no sadness, where even feeling blue is a happy thing. A place inhabited by little blue beings three apples high. It lies deep within an enchanted forest, hidden away beyond the medieval village. Most people believe this place is made up, only to be found in books or children's imagination. Well, we beg to differ."
- - Narrator at the beginning of the movie
"I am not obsessed with Smurfs, thank you; I simply can't stop thinking about the miserable beasts every single minute of every single day! Because I need them! It's only by capturing the little wretches and extracting their happy blue essence that my magic will finally become... not infallible..."
"Meow!"
"INVINCIBLE, yes, thank you! I shall become the most powerful wizard in all of the world!"
[Gargamel and Azrael cackle]
"Yeah, but you're milking it. Don't milk it."
- - Gargamel and Azrael
"Oh, yes... a bit small, but it should do nicely! Oh, it's even got its own cauldron!" [Tries some magic, and screams... ] "OPEN! OPEN! OPEN! OPEN! OPEN! OPPEEENNNN!" [Finally falls out] "Somebody's been working in dark and terrible magic in there!"
- - Gargamel when he mistakes a port-a-potty booth for a laboratory
"Grace, we're being attacked! Do not be fooled by their cuteness!"
- - Patrick Winslow when he gets hog-tied by the Smurfs.
"To review, you guys come from a magic forest where you live in oversized mushrooms..."
"Yes."
"...and you're being chased by an evil wizard..."
"Yeah."
"...and you're trapped in New York until there's a blue moon..."
"Very good."
"...and you like to use the extremely imprecise term 'smurf' for just about everything."
"Smurf-xactly!"
- - Patrick Winslow, Papa Smurf, and Brainy
"And you're all named after your personalities? Do you get your names when you're born or after you've exhibited certain traits?"
[All together] "Yes."
- - Patrick Winslow and the Smurfs
"Whoa, just what is this magic searching device?"
"Right now, I'm using Google."
[All together] "Oooooh...Google."
- - Brainy, Patrick Winslow, and the Smurfs
"None of you finds that song just the tiniest bit annoying?"
"I find it annoying!"
- - Patrick Winslow and Grouchy commenting on the Smurf song
"You guys drink coffee?"
"Is a Smurf's butt blue?"
- - Patrick Winslow and Papa Smurf
"Stop saying 'smurf' for everything! What does that even mean? Smurf! Smurfitty-smurf-smurf-smurf!"
(All the Smurfs gasp)
"There's no call for that kind of language, laddie!"
- - Patrick Winslow and Gutsy
"Are you dead?"
- - Gargamel's constant line to Azrael throughout the movie, later used by Azrael in cat talk when his master gets hit by a bus
"And so the Smurfs left this great city of New York. And I think they left it a little sweeter, a little wiser, a little smurfier. And as that portal began to close for the last time..."
"Hey! Seriously, stop!"
- - Narrator and Grouchy as they re-enter the portal
"Smurfs... Smurfs... I wish I could quit you, get out of here..." (Notices the fourth wall) "What are you looking at?"
- - Gargamel during the end credits