This category features articles about episodes in the Smurfs cartoon show that focus on a character that appeared for only one episode.
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- Sassette's Bewitching Friendship
- Scarlet Croaker (episode)
- Sideshow Smurfs
- Sing A Song Of Smurflings
- Sir Hefty
- Sky High Surprise
- Small Minded Smurfs
- Smurf A Mile In My Shoes
- Smurf To the Future!
- Smurfette's Flower
- Smurfette's Lucky Star
- Smurfs At Sea
- Snappy's Puppet
- Squeaky (episode)
- Sweepy Smurf (episode)
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- The Grouchiest Game In Town
- The Grumpy Gremlin
- The Littlest Giant
- The Lost City Of Yore (episode)
- The Magic Fountain
- The Magical Meanie
- The Patchwork Bear
- The Pluffs!
- The Sand Witch
- The Smurf Odyssey
- The Smurf Who Couldn't Say No
- The Smurf Who Would Be King
- The Smurflings' Unsmurfy Friend
- The Smurfs Of The Round Table
- The Smurfs' Christmas Special
- The Traveler (episode)
- To Smurf A Thief